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arXiv:2005.05811cond-mat.mes-hall

Organic single-photon switch

Anton Zasedatelev, Anton V. Baranikov, Denis Sannikov, Darius Urbonas, Fabio Scafirimuto, Vladislav Yu. Shishkov, Evgeny S. Andrianov, Yurii E. Lozovik, Ullrich Scherf, Thilo Stöferle, Rainer F. Mahrt, Pavlos G. Lagoudakis

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Abstract

The recent progress in nanotechnology [1,2] and single-molecule spectroscopy [3-5] paves the way for cost-effective organic quantum optical technologies emergent with a promise to real-life devices operating at ambient conditions. In this letter, we harness $π$-conjugated segments of an organic ladder-type polymer strongly coupled to a microcavity forming correlated collective dressed states of light, so-called of exciton-polariton condensates. We explore an efficient way for all-optical ultra-fast control over the macroscopic condensate wavefunction via a single photon. Obeying Bose statistics, exciton-polaritons exhibit an extreme nonlinearity undergoing bosonic stimulation [6] which we have managed to trigger at the single-photon level. Relying on the nature of organic matter to sustain stable excitons dressed with high energy molecular vibrations we have developed a principle that allows for single-photon nonlinearity operation at ambient conditions opening the door for practical implementations like sub-picosecond switching, amplification and all-optical logic at the fundamental limit of single light quanta.

arXiv comments
Journal reference
DOI
Subjects
cond-mat.mes-hallMesoscale and Nanoscale Physics physics.opticsOptics quant-phQuantum Physics

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    • I *think* this is a recent-ish preprint of the same paper they're talking about. (The current Nature version is neither open-access nor accessible on Sci-Hub). https://arxiv.org/abs/2005.05811 (E.g., both papers contain this [0] text string pointing to the same URI. But, the…

      perihelionsView on HNParent context

    • If you lack access to it, there's a draft preprint on the arXiv, https://arxiv.org/abs/2005.05811

      perihelionsView on HNParent context

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